Self-Nitrogen-Doped Carbon from Plant Waste as an Oxygen Electrode Material with Exceptional Capacity and Cycling Stability for Lithium-Oxygen Batteries.
Identifieur interne : 000C83 ( Main/Exploration ); précédent : 000C82; suivant : 000C84Self-Nitrogen-Doped Carbon from Plant Waste as an Oxygen Electrode Material with Exceptional Capacity and Cycling Stability for Lithium-Oxygen Batteries.
Auteurs : Meiling Wang [République populaire de Chine] ; Ying Yao [République populaire de Chine] ; Zhenwu Tang [République populaire de Chine] ; Tuo Zhao [République populaire de Chine] ; Feng Wu [République populaire de Chine] ; Yufei Yang [République populaire de Chine] ; Qifei Huang [République populaire de Chine]Source :
- ACS applied materials & interfaces [ 1944-8252 ] ; 2018.
Abstract
To promote the development of electric automobiles, high energy density and high-power batteries are urgently needed. More and more attention has been paid to look for high-performance cathode catalysts for Li-O2 batteries. However, the sluggish kinetic reaction, the stacking of electrical insulation product of Li2O2, and the undesired parasitic reaction restrict their capacity and present poor cycling performance. Here, we prepared nitrogen self-doped activated carbons (N-PIACs) derived from the plant waste (poplar inflorescence) through the activation and slow pyrolysis carbonization method, exhibiting several advantages. The materials presented a three-dimensional interconnecting pore structure and a high surface area. Besides, defects and functional groups doped by nitrogen as active sites improved electrochemical catalysis activity. The Li∥N-PIACs-O2 battery delivered a high specific capacity of 12060 mAh/g, which was 2.3 times that of the pristine plant waste-based Li-O2 battery (N-PICs). In addition, it presented more excellent cycling stability than other common carbon materials. In this study, we developed a functional carbon nanomaterial from cheap natural materials, which might become a highly attractive subject, indicating that this strategy could strengthen the properties of Li-O2 batteries.
DOI: 10.1021/acsami.8b11282
PubMed: 30156825
Affiliations:
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Science and Engineering, School of Materials Science & Engineering , Beijing Institute of Technology , Beijing 100081 </wicri:regionArea><wicri:noRegion>Beijing 100081 </wicri:noRegion></affiliation></author><author><name sortKey="Yao, Ying" sort="Yao, Ying" uniqKey="Yao Y" first="Ying" last="Yao">Ying Yao</name><affiliation wicri:level="1"><nlm:affiliation>Beijing Key Laboratory of Environmental Science and Engineering, School of Materials Science & Engineering , Beijing Institute of Technology , Beijing 100081 , China.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>Beijing Key Laboratory of Environmental Science and Engineering, School of Materials Science & Engineering , Beijing Institute of Technology , Beijing 100081 </wicri:regionArea><wicri:noRegion>Beijing 100081 </wicri:noRegion></affiliation></author><author><name sortKey="Tang, Zhenwu" sort="Tang, Zhenwu" uniqKey="Tang Z" first="Zhenwu" last="Tang">Zhenwu 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100081 </wicri:regionArea><wicri:noRegion>Beijing 100081 </wicri:noRegion></affiliation></author><author><name sortKey="Wu, Feng" sort="Wu, Feng" uniqKey="Wu F" first="Feng" last="Wu">Feng Wu</name><affiliation wicri:level="1"><nlm:affiliation>Beijing Key Laboratory of Environmental Science and Engineering, School of Materials Science & Engineering , Beijing Institute of Technology , Beijing 100081 , China.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>Beijing Key Laboratory of Environmental Science and Engineering, School of Materials Science & Engineering , Beijing Institute of Technology , Beijing 100081 </wicri:regionArea><wicri:noRegion>Beijing 100081 </wicri:noRegion></affiliation></author><author><name sortKey="Yang, Yufei" sort="Yang, Yufei" uniqKey="Yang Y" first="Yufei" last="Yang">Yufei Yang</name><affiliation wicri:level="1"><nlm:affiliation>State Key Laboratory of Environmental Criteria and Risk Assessment , Chinese 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</wicri:noRegion></affiliation></author></analytic><series><title level="j">ACS applied materials & interfaces</title><idno type="eISSN">1944-8252</idno><imprint><date when="2018" type="published">2018</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">To promote the development of electric automobiles, high energy density and high-power batteries are urgently needed. More and more attention has been paid to look for high-performance cathode catalysts for Li-O<sub>2</sub> batteries. However, the sluggish kinetic reaction, the stacking of electrical insulation product of Li<sub>2</sub>O<sub>2</sub>, and the undesired parasitic reaction restrict their capacity and present poor cycling performance. Here, we prepared nitrogen self-doped activated carbons (N-PIACs) derived from the plant waste (poplar inflorescence) through the activation and slow pyrolysis carbonization method, exhibiting several advantages. The materials presented a three-dimensional interconnecting pore structure and a high surface area. Besides, defects and functional groups doped by nitrogen as active sites improved electrochemical catalysis activity. The Li∥N-PIACs-O<sub>2</sub> battery delivered a high specific capacity of 12060 mAh/g, which was 2.3 times that of the pristine plant waste-based Li-O<sub>2</sub> battery (N-PICs). In addition, it presented more excellent cycling stability than other common carbon materials. In this study, we developed a functional carbon nanomaterial from cheap natural materials, which might become a highly attractive subject, indicating that this strategy could strengthen the properties of Li-O<sub>2</sub> batteries.</div></front></TEI><pubmed><MedlineCitation Status="PubMed-not-MEDLINE" Owner="NLM"><PMID Version="1">30156825</PMID><DateCompleted><Year>2018</Year><Month>09</Month><Day>28</Day></DateCompleted><DateRevised><Year>2018</Year><Month>10</Month><Day>01</Day></DateRevised><Article PubModel="Print-Electronic"><Journal><ISSN IssnType="Electronic">1944-8252</ISSN><JournalIssue CitedMedium="Internet"><Volume>10</Volume><Issue>38</Issue><PubDate><Year>2018</Year><Month>Sep</Month><Day>26</Day></PubDate></JournalIssue><Title>ACS applied materials & interfaces</Title><ISOAbbreviation>ACS Appl Mater Interfaces</ISOAbbreviation></Journal><ArticleTitle>Self-Nitrogen-Doped Carbon from Plant Waste as an Oxygen Electrode Material with Exceptional Capacity and Cycling Stability for Lithium-Oxygen Batteries.</ArticleTitle><Pagination><MedlinePgn>32212-32219</MedlinePgn></Pagination><ELocationID EIdType="doi" ValidYN="Y">10.1021/acsami.8b11282</ELocationID><Abstract><AbstractText>To promote the development of electric automobiles, high energy density and high-power batteries are urgently needed. More and more attention has been paid to look for high-performance cathode catalysts for Li-O<sub>2</sub> batteries. However, the sluggish kinetic reaction, the stacking of electrical insulation product of Li<sub>2</sub>O<sub>2</sub>, and the undesired parasitic reaction restrict their capacity and present poor cycling performance. Here, we prepared nitrogen self-doped activated carbons (N-PIACs) derived from the plant waste (poplar inflorescence) through the activation and slow pyrolysis carbonization method, exhibiting several advantages. The materials presented a three-dimensional interconnecting pore structure and a high surface area. Besides, defects and functional groups doped by nitrogen as active sites improved electrochemical catalysis activity. The Li∥N-PIACs-O<sub>2</sub> battery delivered a high specific capacity of 12060 mAh/g, which was 2.3 times that of the pristine plant waste-based Li-O<sub>2</sub> battery (N-PICs). In addition, it presented more excellent cycling stability than other common carbon materials. In this study, we developed a functional carbon nanomaterial from cheap natural materials, which might become a highly attractive subject, indicating that this strategy could strengthen the properties of Li-O<sub>2</sub> batteries.</AbstractText></Abstract><AuthorList CompleteYN="Y"><Author ValidYN="Y"><LastName>Wang</LastName><ForeName>Meiling</ForeName><Initials>M</Initials><AffiliationInfo><Affiliation>Beijing Key Laboratory of Environmental Science and Engineering, School of Materials Science & Engineering , Beijing Institute of Technology , Beijing 100081 , China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Yao</LastName><ForeName>Ying</ForeName><Initials>Y</Initials><Identifier Source="ORCID">http://orcid.org/0000-0002-0472-0852</Identifier><AffiliationInfo><Affiliation>Beijing Key Laboratory of Environmental Science and Engineering, School of Materials Science & Engineering , Beijing Institute of Technology , Beijing 100081 , China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Tang</LastName><ForeName>Zhenwu</ForeName><Initials>Z</Initials><Identifier Source="ORCID">http://orcid.org/0000-0001-6675-791X</Identifier><AffiliationInfo><Affiliation>College of Life and Environmental Sciences , Minzu University of China , Beijing 100081 , China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Zhao</LastName><ForeName>Tuo</ForeName><Initials>T</Initials><AffiliationInfo><Affiliation>Beijing Key Laboratory of Environmental Science and Engineering, School of Materials Science & Engineering , Beijing Institute of Technology , Beijing 100081 , China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Wu</LastName><ForeName>Feng</ForeName><Initials>F</Initials><AffiliationInfo><Affiliation>Beijing Key Laboratory of Environmental Science and Engineering, School of Materials Science & Engineering , Beijing Institute of Technology , Beijing 100081 , China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Yang</LastName><ForeName>Yufei</ForeName><Initials>Y</Initials><AffiliationInfo><Affiliation>State Key Laboratory of Environmental Criteria and Risk Assessment , Chinese Research Academy of Environmental Sciences , Beijing 100012 , China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Huang</LastName><ForeName>Qifei</ForeName><Initials>Q</Initials><AffiliationInfo><Affiliation>State Key Laboratory of Environmental Criteria and Risk Assessment , Chinese Research Academy of Environmental Sciences , Beijing 100012 , China.</Affiliation></AffiliationInfo></Author></AuthorList><Language>eng</Language><PublicationTypeList><PublicationType UI="D016428">Journal Article</PublicationType></PublicationTypeList><ArticleDate DateType="Electronic"><Year>2018</Year><Month>09</Month><Day>14</Day></ArticleDate></Article><MedlineJournalInfo><Country>United States</Country><MedlineTA>ACS Appl Mater Interfaces</MedlineTA><NlmUniqueID>101504991</NlmUniqueID><ISSNLinking>1944-8244</ISSNLinking></MedlineJournalInfo><KeywordList Owner="NOTNLM"><Keyword MajorTopicYN="N">catalyst</Keyword><Keyword MajorTopicYN="N">lithium−oxygen batteries</Keyword><Keyword MajorTopicYN="N">oxygen electrode</Keyword><Keyword MajorTopicYN="N">plant waste</Keyword><Keyword MajorTopicYN="N">self-nitrogen-doped carbon</Keyword></KeywordList></MedlineCitation><PubmedData><History><PubMedPubDate PubStatus="pubmed"><Year>2018</Year><Month>8</Month><Day>30</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="medline"><Year>2018</Year><Month>8</Month><Day>30</Day><Hour>6</Hour><Minute>1</Minute></PubMedPubDate><PubMedPubDate PubStatus="entrez"><Year>2018</Year><Month>8</Month><Day>30</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate></History><PublicationStatus>ppublish</PublicationStatus><ArticleIdList><ArticleId IdType="pubmed">30156825</ArticleId><ArticleId IdType="doi">10.1021/acsami.8b11282</ArticleId></ArticleIdList></PubmedData></pubmed><affiliations><list><country><li>République populaire de Chine</li></country></list><tree><country name="République populaire de Chine"><noRegion><name sortKey="Wang, Meiling" sort="Wang, Meiling" uniqKey="Wang M" first="Meiling" last="Wang">Meiling Wang</name></noRegion><name sortKey="Huang, Qifei" sort="Huang, Qifei" uniqKey="Huang Q" first="Qifei" last="Huang">Qifei Huang</name><name sortKey="Tang, Zhenwu" sort="Tang, Zhenwu" uniqKey="Tang Z" first="Zhenwu" last="Tang">Zhenwu Tang</name><name sortKey="Wu, Feng" sort="Wu, Feng" uniqKey="Wu F" first="Feng" last="Wu">Feng Wu</name><name sortKey="Yang, Yufei" sort="Yang, Yufei" uniqKey="Yang Y" first="Yufei" last="Yang">Yufei Yang</name><name sortKey="Yao, Ying" sort="Yao, Ying" uniqKey="Yao Y" first="Ying" last="Yao">Ying Yao</name><name sortKey="Zhao, Tuo" sort="Zhao, Tuo" uniqKey="Zhao T" first="Tuo" last="Zhao">Tuo Zhao</name></country></tree></affiliations></record>Pour manipuler ce document sous Unix (Dilib)
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